How it Works
Rubber elasticity arises from the entropic elasticity of cross-linked polymer chains. At rest, chains adopt random-coil configurations with maximum entropy. Stretching reduces chain entropy, and the Gaussian statistics of random walks gives a linear restoring force per chain. Summing over all network strands gives the macroscopic stress-stretch relation.
Three constitutive models are shown: Neo-Hookean (simplest, one parameter G), Mooney-Rivlin (two parameters C₁, C₂, better for moderate strains), and Gent (accounts for finite extensibility through Jₘ, the maximum value of I₁ - 3, causing stress to diverge at limiting stretch).
Mooney-Rivlin: σ = 2(C₁ + C₂·λ⁻¹)·(λ − λ⁻²)
Gent: σ = G·(λ − λ⁻²)·Jₘ / [Jₘ − (λ² + 2λ⁻¹ − 3)]
I₁ = λ² + 2λ⁻¹ (first invariant, uniaxial)
Frequently Asked Questions
What is rubber elasticity?
Rubber elasticity is the large, reversible deformation behavior of cross-linked polymer networks. Unlike metals, rubber elasticity is entropic in origin: stretching reduces the conformational entropy of polymer chains, and the restoring force is an entropic spring.
What is the neo-Hookean model?
The neo-Hookean model gives stress as σ = G(λ - λ⁻²) for uniaxial tension, where G = nkT is the shear modulus, n is the cross-link density, k is Boltzmann's constant, T is temperature, and λ is the stretch ratio.
What is the stretch ratio λ?
The stretch ratio λ = L/L₀ is the ratio of deformed length to original length. For incompressible rubber, uniaxial stretching (λ > 1) causes lateral contraction with λ_y = λ_z = λ⁻¹/². Engineering strain ε = λ − 1.
What is the Mooney-Rivlin model?
Mooney-Rivlin extends neo-Hookean by adding a second invariant term: σ = 2(C₁ + C₂/λ)(λ - λ⁻²). The Mooney plot of σ/2(λ - λ⁻²) vs 1/λ gives a straight line with slope C₂ and intercept C₁. It better fits real rubber at moderate stretches.
What is the Gent model?
The Gent model accounts for the finite extensibility of polymer chains via parameter Jₘ. As λ approaches the limiting stretch, stress diverges, mimicking strain stiffening observed in real rubber networks.
Why does G = nkT?
From statistical mechanics of Gaussian chains, each network strand stores entropic energy proportional to kT. Summing over n network strands per unit volume gives shear modulus G = nkT. Higher cross-link density leads to higher G.
What is strain-induced crystallization?
At high stretch ratios (λ > 4–6 for natural rubber), polymer chains become aligned and can crystallize, causing an upturn in the stress-strain curve. This greatly increases tear resistance and is why natural rubber outperforms synthetic rubber in many applications.
How does temperature affect rubber modulus?
For ideal rubber elasticity, G = nkT, so modulus increases linearly with absolute temperature. This thermo-elastic inversion (rubber stiffens on heating) contrasts with metals that soften. At very low T, rubber undergoes glass transition and becomes rigid.
What is the Mullins effect?
The Mullins effect is stress-softening observed in filled rubbers after the first large deformation. Reloading follows a lower stress path than the first loading. It is attributed to rupture of filler-polymer bonds and is partially recovered upon heating.
What are common cross-linking methods for rubber?
Vulcanization with sulfur (natural rubber) creates polysulfide bridges. Peroxide cross-linking creates carbon-carbon bonds for better heat resistance. Radiation cross-linking is used for silicone and polyethylene. Cross-link density controls hardness and modulus.